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Measurements of the Carrier Dynamics and Terahertz Response of Oriented Germanium Nanowires using Optical-Pump Terahertz-Probe Spectroscopy

机译:面向对象的载流子动力学和太赫兹响应的测量   锗纳米线使用光泵太赫兹探针光谱

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摘要

We have measured the terahertz response of oriented germanium nanowires usingultrafast optical-pump terahertz-probe spectroscopy. We present results on thetime, frequency, and polarization dependence of the terahertz response. Ourresults indicate intraband energy relaxation times of photoexcited carriers inthe 1.5-2.0 ps range, carrier density dependent interband electron-holerecombination times in the 75-125 ps range, and carrier momentum scatteringrates in the 60-90 fs range. Additionally, the terahertz response of thenanowires is strongly polarization dependent despite the subwavelengthdimensions of the nanowires. The differential terahertz transmission is foundto be large when the field is polarized parallel to the nanowires and verysmall when the field is polarized perpendicular to the nanowires. Thispolarization dependence of the terahertz response can be explained in terms ofthe induced depolarization fields and the resulting magnitudes of the surfaceplasmon frequencies.
机译:我们已经使用超快光泵太赫兹-探针光谱法测量了取向锗纳米线的太赫兹响应。我们提出了关于太赫兹响应的时间,频率和极化相关性的结果。我们的结果表明,光激发载流子的带内能量弛豫时间在1.5-2.0 ps范围内,依赖于载流子密度的带内电子-空穴复合时间在75-125 ps范围内,载流子动量散射率在60-90 fs范围内。另外,尽管纳米线的子波长尺寸较大,然后纳米线的太赫兹响应仍强烈依赖偏振。发现当电场平行于纳米线极化时,差分太赫兹透射很大,而当电场垂直于纳米线极化时,差分太赫兹透射很小。太赫兹响应的这种极化依赖性可以通过感应的去极化场和由此产生的表面等离激元频率幅度来解释。

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